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Add blueberries and 1/4 cup limoncello to a high speed blender or food processor and puree until smooth
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Pour into popsicle molds 1/3 full
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Rinse blender and add strawberries and remaining 1/4 cup limoncello and puree until smooth
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Slowly pour coconut milk on top of blueberry popsicle layer to 2/3 full
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Slowly pour the strawberry limoncello puree on top of the coconut milk layer to fill the molds
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Cover, insert sticks, and freeze overnight